Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity

We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth's atmospheric methane concentration (CCH4) and its isotope ratio δ13CH4 over the last four decades. We identify oscillations between positive and negative feedbacks, show...

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Main Authors: Cheng, Chin-Hsien, Redfern, Simon Anthony Turner
Other Authors: Asian School of the Environment
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/168648
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spelling sg-ntu-dr.10356-1686482023-06-19T15:30:48Z Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity Cheng, Chin-Hsien Redfern, Simon Anthony Turner Asian School of the Environment School of Materials Science and Engineering Science::Geology Air Temperature Annual Variation We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth's atmospheric methane concentration (CCH4) and its isotope ratio δ13CH4 over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing CCH4. Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing CCH4 due to weakened methane sink via atmospheric •OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when CCH4 is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when •OH is limiting, negative feedback is favoured. Incorporating the interannually increasing CCH4 via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m-2 °C-1, much higher than the IPCC AR6 estimate. Nanyang Technological University Published version This work was supported by NTU Singapore’s start-up grant to SATR. 2023-06-13T05:02:34Z 2023-06-13T05:02:34Z 2022 Journal Article Cheng, C. & Redfern, S. A. T. (2022). Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity. Nature Communications, 13(1), 3592-. https://dx.doi.org/10.1038/s41467-022-31345-w 2041-1723 https://hdl.handle.net/10356/168648 10.1038/s41467-022-31345-w 35739128 2-s2.0-85132685567 1 13 3592 en Nature Communications © 2022 The Author(s). This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Geology
Air Temperature
Annual Variation
spellingShingle Science::Geology
Air Temperature
Annual Variation
Cheng, Chin-Hsien
Redfern, Simon Anthony Turner
Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
description We estimate the causal contributions of spatiotemporal changes in temperature (T) and precipitation (Pr) to changes in Earth's atmospheric methane concentration (CCH4) and its isotope ratio δ13CH4 over the last four decades. We identify oscillations between positive and negative feedbacks, showing that both contribute to increasing CCH4. Interannually, increased emissions via positive feedbacks (e.g. wetland emissions and wildfires) with higher land surface air temperature (LSAT) are often followed by increasing CCH4 due to weakened methane sink via atmospheric •OH, via negative feedbacks with lowered sea surface temperatures (SST), especially in the tropics. Over decadal time scales, we find alternating rate-limiting factors for methane oxidation: when CCH4 is limiting, positive methane-climate feedback via direct oceanic emissions dominates; when •OH is limiting, negative feedback is favoured. Incorporating the interannually increasing CCH4 via negative feedbacks gives historical methane-climate feedback sensitivity ≈ 0.08 W m-2 °C-1, much higher than the IPCC AR6 estimate.
author2 Asian School of the Environment
author_facet Asian School of the Environment
Cheng, Chin-Hsien
Redfern, Simon Anthony Turner
format Article
author Cheng, Chin-Hsien
Redfern, Simon Anthony Turner
author_sort Cheng, Chin-Hsien
title Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_short Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_full Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_fullStr Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_full_unstemmed Impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
title_sort impact of interannual and multidecadal trends on methane-climate feedbacks and sensitivity
publishDate 2023
url https://hdl.handle.net/10356/168648
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