Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces

We present a new approach to achieving strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface. Here a high-finesse metasurface cavity is monolithically patterned in the channel of a perovskite light-emitting transistor to induce...

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Main Authors: Wang, Yutao, Tian, Jingyi, Klein, Maciej, Adamo, Giorgio, Ha, Son Tung, Soci, Cesare
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/170323
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Institution: Nanyang Technological University
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spelling sg-ntu-dr.10356-1703232024-07-22T15:34:35Z Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces Wang, Yutao Tian, Jingyi Klein, Maciej Adamo, Giorgio Ha, Son Tung Soci, Cesare School of Physical and Mathematical Sciences Interdisciplinary Graduate School (IGS) Centre for Disruptive Photonic Technologies (CDPT) The Photonics Institute Energy Research Institute @ NTU (ERI@N) Physics Dielectric Metasurfaces Light-emitting Transistor We present a new approach to achieving strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface. Here a high-finesse metasurface cavity is monolithically patterned in the channel of a perovskite light-emitting transistor to induce a large Rabi splitting of ∼200 meV and more than 50-fold enhancement of the polaritonic emission compared to the intrinsic excitonic emission of the perovskite film. Moreover, the directionality of polaritonic electroluminescence can be dynamically tuned by varying the source-drain bias, which induces an asymmetric distribution of exciton population within the transistor channel. We argue that this approach provides a new platform to study strong light-matter interactions in dispersion engineered photonic cavities under electrical injection and paves the way to solution-processed electrically pumped polariton lasers. Agency for Science, Technology and Research (A*STAR) Ministry of Education (MOE) Submitted/Accepted version Research was supported by the Agency for Science, Technology and Research (A*STAR-AME programmatic grant on Nanoantenna Spatial Light Modulators for Next-Gen Display Technologies, grant no. A18A7b0058) and the Singapore Ministry of Education (grant no. MOE2016-T3-1-006). S.T.H. acknowledges support from AME Young Individual Research Grant (YIRG grant no. A2084c0177) and A*STAR MTC-Programmatic Fund (grant no. M21J9b0085). 2023-09-07T02:44:02Z 2023-09-07T02:44:02Z 2023 Journal Article Wang, Y., Tian, J., Klein, M., Adamo, G., Ha, S. T. & Soci, C. (2023). Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces. Nano Letters, 23(10), 4431-4438. https://dx.doi.org/10.1021/acs.nanolett.3c00727 1530-6984 https://hdl.handle.net/10356/170323 10.1021/acs.nanolett.3c00727 37129264 2-s2.0-85159592864 10 23 4431 4438 en A18A7b0058 MOE2016-T3-1-006 A2084c0177 M21J9b0085 Nano Letters 10.21979/N9/866ZPH © 2023 American Chemical Society. All rights reserved. This article may be downloaded for personal use only. Any other use requires prior permission of the copyright holder. The Version of Record is available online at http://doi.org/10.1021/acs.nanolett.3c00727. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Physics
Dielectric Metasurfaces
Light-emitting Transistor
spellingShingle Physics
Dielectric Metasurfaces
Light-emitting Transistor
Wang, Yutao
Tian, Jingyi
Klein, Maciej
Adamo, Giorgio
Ha, Son Tung
Soci, Cesare
Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
description We present a new approach to achieving strong coupling between electrically injected excitons and photonic bound states in the continuum of a dielectric metasurface. Here a high-finesse metasurface cavity is monolithically patterned in the channel of a perovskite light-emitting transistor to induce a large Rabi splitting of ∼200 meV and more than 50-fold enhancement of the polaritonic emission compared to the intrinsic excitonic emission of the perovskite film. Moreover, the directionality of polaritonic electroluminescence can be dynamically tuned by varying the source-drain bias, which induces an asymmetric distribution of exciton population within the transistor channel. We argue that this approach provides a new platform to study strong light-matter interactions in dispersion engineered photonic cavities under electrical injection and paves the way to solution-processed electrically pumped polariton lasers.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Wang, Yutao
Tian, Jingyi
Klein, Maciej
Adamo, Giorgio
Ha, Son Tung
Soci, Cesare
format Article
author Wang, Yutao
Tian, Jingyi
Klein, Maciej
Adamo, Giorgio
Ha, Son Tung
Soci, Cesare
author_sort Wang, Yutao
title Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
title_short Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
title_full Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
title_fullStr Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
title_full_unstemmed Directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
title_sort directional emission from electrically injected exciton-polaritons in perovskite metasurfaces
publishDate 2023
url https://hdl.handle.net/10356/170323
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