Multicolor x-rays from free electron-driven van der Waals heterostructures

The emergence of van der Waals (vdW) heterostructures has led to precise and versatile methods of fabricating devices with atomic-scale accuracies. Hence, vdW heterostructures have shown much promise for technologies including photodetectors, photocatalysis, photovoltaic devices, ultrafast photonic...

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Main Authors: Huang, Sunchao, Duan, Ruihuan, Pramanik, Nikhil, Go, Michael, Boothroyd, Chris, Liu, Zheng, Wong, Liang Jie
Other Authors: School of Electrical and Electronic Engineering
Format: Article
Language:English
Published: 2023
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Online Access:https://hdl.handle.net/10356/172743
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1727432023-12-22T15:40:45Z Multicolor x-rays from free electron-driven van der Waals heterostructures Huang, Sunchao Duan, Ruihuan Pramanik, Nikhil Go, Michael Boothroyd, Chris Liu, Zheng Wong, Liang Jie School of Electrical and Electronic Engineering School of Materials Science and Engineering Facility for Analysis, Characterisation, Testing and Simulation CNRS International NTU THALES Research Alliances Science::Physics::Optics and light Electron Beam Field Effect Transistor The emergence of van der Waals (vdW) heterostructures has led to precise and versatile methods of fabricating devices with atomic-scale accuracies. Hence, vdW heterostructures have shown much promise for technologies including photodetectors, photocatalysis, photovoltaic devices, ultrafast photonic devices, and field-effect transistors. These applications, however, remain confined to optical and suboptical regimes. Here, we theoretically show and experimentally demonstrate the use of vdW heterostructures as platforms for multicolor x-ray generation. By driving the vdW heterostructures with free electrons in a table-top setup, we generate x-ray photons whose output spectral profile can be user-customized via the heterostructure design and even controlled in real time. We show that the multicolor photon energies and their corresponding intensities can be tailored by varying the electron energy, the electron beam position, as well as the geometry and composition of the vdW heterostructure. Our results reveal the promise of vdW heterostructures in realizing highly versatile x-ray sources for emerging applications in advanced x-ray imaging and spectroscopy. Ministry of Education (MOE) Nanyang Technological University National Research Foundation (NRF) Published version This research is partially supported by the National Research Foundation, Singapore (Project ID NRF2020-NRF-ISF004-3525) and the Ministry of Education, Singapore, under its AcRF- Tier 2 programme (award no. MOE-T2EP50222-0012). L.J.W. acknowledges the support of the Nanyang Assistant Professorship Start-up Grant. 2023-12-21T04:17:33Z 2023-12-21T04:17:33Z 2023 Journal Article Huang, S., Duan, R., Pramanik, N., Go, M., Boothroyd, C., Liu, Z. & Wong, L. J. (2023). Multicolor x-rays from free electron-driven van der Waals heterostructures. Science Advances, 9(48), eadj8584-. https://dx.doi.org/10.1126/sciadv.adj8584 2375-2548 https://hdl.handle.net/10356/172743 10.1126/sciadv.adj8584 38039369 2-s2.0-85178325791 48 9 eadj8584 en NRF2020-NRF-ISF004-3525 MOE-T2EP50222-0012 NTU-SUG Science Advances © 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 CC BY-NC). application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Science::Physics::Optics and light
Electron Beam
Field Effect Transistor
spellingShingle Science::Physics::Optics and light
Electron Beam
Field Effect Transistor
Huang, Sunchao
Duan, Ruihuan
Pramanik, Nikhil
Go, Michael
Boothroyd, Chris
Liu, Zheng
Wong, Liang Jie
Multicolor x-rays from free electron-driven van der Waals heterostructures
description The emergence of van der Waals (vdW) heterostructures has led to precise and versatile methods of fabricating devices with atomic-scale accuracies. Hence, vdW heterostructures have shown much promise for technologies including photodetectors, photocatalysis, photovoltaic devices, ultrafast photonic devices, and field-effect transistors. These applications, however, remain confined to optical and suboptical regimes. Here, we theoretically show and experimentally demonstrate the use of vdW heterostructures as platforms for multicolor x-ray generation. By driving the vdW heterostructures with free electrons in a table-top setup, we generate x-ray photons whose output spectral profile can be user-customized via the heterostructure design and even controlled in real time. We show that the multicolor photon energies and their corresponding intensities can be tailored by varying the electron energy, the electron beam position, as well as the geometry and composition of the vdW heterostructure. Our results reveal the promise of vdW heterostructures in realizing highly versatile x-ray sources for emerging applications in advanced x-ray imaging and spectroscopy.
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Huang, Sunchao
Duan, Ruihuan
Pramanik, Nikhil
Go, Michael
Boothroyd, Chris
Liu, Zheng
Wong, Liang Jie
format Article
author Huang, Sunchao
Duan, Ruihuan
Pramanik, Nikhil
Go, Michael
Boothroyd, Chris
Liu, Zheng
Wong, Liang Jie
author_sort Huang, Sunchao
title Multicolor x-rays from free electron-driven van der Waals heterostructures
title_short Multicolor x-rays from free electron-driven van der Waals heterostructures
title_full Multicolor x-rays from free electron-driven van der Waals heterostructures
title_fullStr Multicolor x-rays from free electron-driven van der Waals heterostructures
title_full_unstemmed Multicolor x-rays from free electron-driven van der Waals heterostructures
title_sort multicolor x-rays from free electron-driven van der waals heterostructures
publishDate 2023
url https://hdl.handle.net/10356/172743
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