Fifth-Order Three-Dimensional Electronic Spectroscopy Using a Pump–Probe Configuration

• المؤلفون الرئيسيون: Zhang, Zhengyang, Wells, Kym L., Seidel, Marco T., Tan, Howe-Siang
• مؤلفون آخرون: School of Physical and Mathematical Sciences
• التنسيق: مقال
• اللغة: English
• منشور في: 2016
• الموضوعات: Chemistry and Biological Chemistry
• الوصول للمادة أونلاين: https://hdl.handle.net/10356/82240; http://hdl.handle.net/10220/39845
• المؤسسة: Nanyang Technological University

We present the theoretical details and experimental demonstration of fifth-order three-dimensional (3D) electronic spectroscopy using a pump–probe beam geometry. This is achieved using a pulse shaper and appropriate phase cycling schemes. We show how 8-step and 27-step phase cycling schemes can meas...