Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy
Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cyc...
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sg-ntu-dr.10356-961202020-03-07T12:37:05Z Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang School of Physical and Mathematical Sciences Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cycling schemes can be employed to retrieve both rephasing and nonrephasing 2D spectra. The studies were performed on the Qy transition of chlorophyll a. 2013-06-27T06:42:45Z 2019-12-06T19:26:04Z 2013-06-27T06:42:45Z 2019-12-06T19:26:04Z 2012 2012 Journal Article Zhang, Z., Wells, K. L., Hyland, E. W. J., & Tan, H.-S. (2012). Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy. Chemical Physics Letters, 550, 156-161. 0009-2614 https://hdl.handle.net/10356/96120 http://hdl.handle.net/10220/10813 10.1016/j.cplett.2012.08.037 en Chemical physics letters © 2012 Elsevier B.V. |
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Experimental demonstrations and detailed theoretical explanations are provided for a thorough understanding of the various phase-cycling schemes in an optical pulse shaper assisted two-dimensional electronic spectroscopy (2DES) in a pump–probe beam geometry. We show that two and three-step phase-cycling schemes can be employed to retrieve both rephasing and nonrephasing 2D spectra. The studies were performed on the Qy transition of chlorophyll a. |
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School of Physical and Mathematical Sciences |
| author_facet |
School of Physical and Mathematical Sciences Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang |
| format |
Article |
| author |
Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang |
| spellingShingle |
Zhang, Zhengyang Wells, Kym Lewis Hyland, Edward William James Tan, Howe-Siang Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| author_sort |
Zhang, Zhengyang |
| title |
Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_short |
Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_full |
Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_fullStr |
Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_full_unstemmed |
Phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| title_sort |
phase-cycling schemes for pump–probe beam geometry two-dimensional electronic spectroscopy |
| publishDate |
2013 |
| url |
https://hdl.handle.net/10356/96120 http://hdl.handle.net/10220/10813 |
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1681035663951003648 |