Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources

Highly tensile-strained Ge quantum dots (TS-Ge-QDs) emitting structures with different size were successfully grown on InP substrates by molecular beam epitaxy. Defect-free samples with TS-Ge-QDs were confirmed by transmission electron microscopy. Finite element modeling indicates a maximum tensile...

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Main Authors: Chen, Qimiao, Zhang, Liyao, Song, Yuxin, Chen, Xiren, Koelling, Sebastian, Zhang, Zhenpu, Li, Yaoyao, Koenraad, Paul M., Shao, Jun, Tan, Chuan Seng, Wang, Shumin, Gong, Qian
Other Authors: School of Electrical and Electronic Engineering
Format: Article
Language:English
Published: 2021
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Online Access:https://hdl.handle.net/10356/146062
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-1460622021-01-25T01:46:12Z Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources Chen, Qimiao Zhang, Liyao Song, Yuxin Chen, Xiren Koelling, Sebastian Zhang, Zhenpu Li, Yaoyao Koenraad, Paul M. Shao, Jun Tan, Chuan Seng Wang, Shumin Gong, Qian School of Electrical and Electronic Engineering Engineering::Electrical and electronic engineering::Semiconductors GeSn QD Mid-IR Light Source Highly tensile-strained Ge quantum dots (TS-Ge-QDs) emitting structures with different size were successfully grown on InP substrates by molecular beam epitaxy. Defect-free samples with TS-Ge-QDs were confirmed by transmission electron microscopy. Finite element modeling indicates a maximum tensile strain of 4.5% in the Ge QDs, which is much larger than the required strain to achieve direct bandgap conversion of Ge based on theoretical prediction. Photoluminescence (PL) from a direct bandgap-like transition of TS-Ge-QDs with a peak energy of 0.796 eV was achieved and confirmed by the etch depth-dependent PL, temperature-dependent PL and power-dependent PL. In addition, a strong defect-related peak of 1 eV was observed at room temperature. The band structure of the TS-Ge-QDs emitting structures was calculated to support the experimental results of PL spectra. Achieving PL from direct bandgap-like transitions of TS-Ge-QDs provides encouraging evidence of this promising method for integrated light source on Si photonics platform. National Research Foundation (NRF) Accepted version The authors would like to thank the financial support from the National Research Foundation of Singapore under the Competitive Research Program (NRF–CRP19–2017–01) 2021-01-25T01:46:12Z 2021-01-25T01:46:12Z 2021 Journal Article Chen, Q., Zhang, L., Song, Y., Chen, X., Koelling, S., Zhang, Z., ... Gong, Q. (2021). Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources. ACS Applied Nano Materials, 4(1), 897–906. doi:10.1021/acsanm.0c03373 2574-0970 https://hdl.handle.net/10356/146062 10.1021/acsanm.0c03373 1 4 897 906 en ACS Applied Nano Materials This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Applied Nano Materials, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see https://doi.org/10.1021/acsanm.0c03373 application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Electrical and electronic engineering::Semiconductors
GeSn QD
Mid-IR Light Source
spellingShingle Engineering::Electrical and electronic engineering::Semiconductors
GeSn QD
Mid-IR Light Source
Chen, Qimiao
Zhang, Liyao
Song, Yuxin
Chen, Xiren
Koelling, Sebastian
Zhang, Zhenpu
Li, Yaoyao
Koenraad, Paul M.
Shao, Jun
Tan, Chuan Seng
Wang, Shumin
Gong, Qian
Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
description Highly tensile-strained Ge quantum dots (TS-Ge-QDs) emitting structures with different size were successfully grown on InP substrates by molecular beam epitaxy. Defect-free samples with TS-Ge-QDs were confirmed by transmission electron microscopy. Finite element modeling indicates a maximum tensile strain of 4.5% in the Ge QDs, which is much larger than the required strain to achieve direct bandgap conversion of Ge based on theoretical prediction. Photoluminescence (PL) from a direct bandgap-like transition of TS-Ge-QDs with a peak energy of 0.796 eV was achieved and confirmed by the etch depth-dependent PL, temperature-dependent PL and power-dependent PL. In addition, a strong defect-related peak of 1 eV was observed at room temperature. The band structure of the TS-Ge-QDs emitting structures was calculated to support the experimental results of PL spectra. Achieving PL from direct bandgap-like transitions of TS-Ge-QDs provides encouraging evidence of this promising method for integrated light source on Si photonics platform.
author2 School of Electrical and Electronic Engineering
author_facet School of Electrical and Electronic Engineering
Chen, Qimiao
Zhang, Liyao
Song, Yuxin
Chen, Xiren
Koelling, Sebastian
Zhang, Zhenpu
Li, Yaoyao
Koenraad, Paul M.
Shao, Jun
Tan, Chuan Seng
Wang, Shumin
Gong, Qian
format Article
author Chen, Qimiao
Zhang, Liyao
Song, Yuxin
Chen, Xiren
Koelling, Sebastian
Zhang, Zhenpu
Li, Yaoyao
Koenraad, Paul M.
Shao, Jun
Tan, Chuan Seng
Wang, Shumin
Gong, Qian
author_sort Chen, Qimiao
title Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
title_short Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
title_full Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
title_fullStr Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
title_full_unstemmed Highly tensile-strained self-assembled Ge quantum dots on InP substrates for integrated light sources
title_sort highly tensile-strained self-assembled ge quantum dots on inp substrates for integrated light sources
publishDate 2021
url https://hdl.handle.net/10356/146062
_version_ 1690658298902085632