Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses

Ultrathin flat optics allow control of light at the subwavelength scale that is unmatched by traditional refractive optics. To approach the atomically thin limit, the use of 2D materials is an attractive possibility due to their high refractive indices. However, achievement of diffraction-limited fo...

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Main Authors: Lin, Han, Xu, Zai-Quan, Cao, Guiyuan, Zhang, Yupeng, Zhou, Jiadong, Wang, Ziyu, Wan, Zhichen, Liu, Zheng, Loh, Kian Ping, Qiu, Cheng-Wei, Bao, Qiaoliang, Jia, Baohua
Other Authors: School of Materials Science and Engineering
Format: Article
Language:English
Published: 2021
Subjects:
Online Access:https://hdl.handle.net/10356/147278
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Institution: Nanyang Technological University
Language: English
id sg-ntu-dr.10356-147278
record_format dspace
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
topic Engineering::Materials
Micro-optics
Nanoparticles
spellingShingle Engineering::Materials
Micro-optics
Nanoparticles
Lin, Han
Xu, Zai-Quan
Cao, Guiyuan
Zhang, Yupeng
Zhou, Jiadong
Wang, Ziyu
Wan, Zhichen
Liu, Zheng
Loh, Kian Ping
Qiu, Cheng-Wei
Bao, Qiaoliang
Jia, Baohua
Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
description Ultrathin flat optics allow control of light at the subwavelength scale that is unmatched by traditional refractive optics. To approach the atomically thin limit, the use of 2D materials is an attractive possibility due to their high refractive indices. However, achievement of diffraction-limited focusing and imaging is challenged by their thickness-limited spatial resolution and focusing efficiency. Here we report a universal method to transform 2D monolayers into ultrathin flat lenses. Femtosecond laser direct writing was applied to generate local scattering media inside a monolayer, which overcomes the longstanding challenge of obtaining sufficient phase or amplitude modulation in atomically thin 2D materials. We achieved highly efficient 3D focusing with subwavelength resolution and diffraction-limited imaging. The high focusing performance even allows diffraction-limited imaging at different focal positions with varying magnifications. Our work paves the way for downscaling of optical devices using 2D materials and reports an unprecedented approach for fabricating ultrathin imaging devices.
author2 School of Materials Science and Engineering
author_facet School of Materials Science and Engineering
Lin, Han
Xu, Zai-Quan
Cao, Guiyuan
Zhang, Yupeng
Zhou, Jiadong
Wang, Ziyu
Wan, Zhichen
Liu, Zheng
Loh, Kian Ping
Qiu, Cheng-Wei
Bao, Qiaoliang
Jia, Baohua
format Article
author Lin, Han
Xu, Zai-Quan
Cao, Guiyuan
Zhang, Yupeng
Zhou, Jiadong
Wang, Ziyu
Wan, Zhichen
Liu, Zheng
Loh, Kian Ping
Qiu, Cheng-Wei
Bao, Qiaoliang
Jia, Baohua
author_sort Lin, Han
title Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
title_short Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
title_full Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
title_fullStr Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
title_full_unstemmed Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses
title_sort diffraction-limited imaging with monolayer 2d material-based ultrathin flat lenses
publishDate 2021
url https://hdl.handle.net/10356/147278
_version_ 1773551237523832832
spelling sg-ntu-dr.10356-1472782023-07-14T16:01:48Z Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses Lin, Han Xu, Zai-Quan Cao, Guiyuan Zhang, Yupeng Zhou, Jiadong Wang, Ziyu Wan, Zhichen Liu, Zheng Loh, Kian Ping Qiu, Cheng-Wei Bao, Qiaoliang Jia, Baohua School of Materials Science and Engineering Engineering::Materials Micro-optics Nanoparticles Ultrathin flat optics allow control of light at the subwavelength scale that is unmatched by traditional refractive optics. To approach the atomically thin limit, the use of 2D materials is an attractive possibility due to their high refractive indices. However, achievement of diffraction-limited focusing and imaging is challenged by their thickness-limited spatial resolution and focusing efficiency. Here we report a universal method to transform 2D monolayers into ultrathin flat lenses. Femtosecond laser direct writing was applied to generate local scattering media inside a monolayer, which overcomes the longstanding challenge of obtaining sufficient phase or amplitude modulation in atomically thin 2D materials. We achieved highly efficient 3D focusing with subwavelength resolution and diffraction-limited imaging. The high focusing performance even allows diffraction-limited imaging at different focal positions with varying magnifications. Our work paves the way for downscaling of optical devices using 2D materials and reports an unprecedented approach for fabricating ultrathin imaging devices. Agency for Science, Technology and Research (A*STAR) National Research Foundation (NRF) Published version B. J. acknowledges support from the Australian Research Council through the Discovery Project scheme (DP190103186) and the Industrial Transformation Training Centres scheme (Grant No. IC180100005). Z.-Q. X. acknowledges support from the Australian Postgraduate Award (APA) and international postgraduate research scholarship (IPRS). Y. Z. acknowledges support from the National Key Research & Development Program (No. 2016YFA0201902) and Shenzhen Nanshan District Pilotage Team Program (LHTD20170006). Q. B. acknowledges support from the Australian Research Council (FT150100450 and CE170100039). C.-W. Q. acknowledges financial support from the A*STAR Pharos Program (grant number 15270 00014, with project number R-263–000-B91–305) and the National Research Foundation, Prime Minister’s Office, Singapore under its Competitive Research Program (CRP award NRF CRP22–2019–0006). Z. L. acknowledges the support of the National Research Foundation–Competitive Research Program (NRF-CRP21–2018–007). This work was performed in part at the Melbourne Centre for Nanofabrication (MCN) in the Victorian Node of the Australian National Fabrication Facility (ANFF). The authors would like to thank Yu-Han Wang and Wei-Yen Woon and Professor Chia Hao Chen for their assistance with scanning XPS (X-ray photoelectron spectroscopy) measurements. The authors also acknowledge the Swinburne Laser Nanofabrication Facility for support in device fabrication and characterization. 2021-03-26T07:11:28Z 2021-03-26T07:11:28Z 2020 Journal Article Lin, H., Xu, Z., Cao, G., Zhang, Y., Zhou, J., Wang, Z., Wan, Z., Liu, Z., Loh, K. P., Qiu, C., Bao, Q. & Jia, B. (2020). Diffraction-limited imaging with monolayer 2D material-based ultrathin flat lenses. Light: Science and Applications, 9(1). https://dx.doi.org/10.1038/s41377-020-00374-9 2095-5545 0000-0002-6262-1959 0000-0001-7291-1426 0000-0002-8825-7198 0000-0002-1491-743X 0000-0002-6605-500X 0000-0002-6971-789X 0000-0002-6703-477X https://hdl.handle.net/10356/147278 10.1038/s41377-020-00374-9 32821378 2-s2.0-85089385514 1 9 en NRF-CRP22–2019–0006 R-263–000-B91–305 NRF-CRP21–2018–007 Light: Science and Applications © 2020 The Author(s). This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license,and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. application/pdf