Purely absorptive fifth-order three-dimensional electronic spectroscopy

Purely absorptive fifth-order three-dimensional electronic spectroscopy

We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data proce...

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Main Authors: Zhang, Zhengyang, Wells, Kym Lewis, Tan, Howe-Siang
Other Authors: School of Physical and Mathematical Sciences
Format: Article
Language:English
Published: 2013
Online Access:https://hdl.handle.net/10356/99325
http://hdl.handle.net/10220/10942
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Institution: Nanyang Technological University
Language: English
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spelling sg-ntu-dr.10356-993252023-02-28T19:36:47Z Purely absorptive fifth-order three-dimensional electronic spectroscopy Zhang, Zhengyang Wells, Kym Lewis Tan, Howe-Siang School of Physical and Mathematical Sciences We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data processing, purely absorptive 3D spectra of chlorophyll a are obtained. Published version 2013-07-04T03:36:21Z 2019-12-06T20:05:57Z 2013-07-04T03:36:21Z 2019-12-06T20:05:57Z 2012 2012 Journal Article Zhang, Z., Wells, K., & Tan, H.-S. (2012). Purely absorptive fifth-order three-dimensional electronic spectroscopy. Optics Letters, 37(24), 5058-5060. 0146-9592 https://hdl.handle.net/10356/99325 http://hdl.handle.net/10220/10942 10.1364/OL.37.005058 en Optics letters © 2012 Optical Society of America. This paper was published in Optics Letters and is made available as an electronic reprint (preprint) with permission of Optical Society of America. The paper can be found at the following official DOI: [http://dx.doi.org/10.1364/OL.37.005058]. One print or electronic copy may be made for personal use only. Systematic or multiple reproduction, distribution to multiple locations via electronic or other means, duplication of any material in this paper for a fee or for commercial purposes, or modification of the content of the paper is prohibited and is subject to penalties under law. application/pdf
institution Nanyang Technological University
building NTU Library
continent Asia
country Singapore
Singapore
content_provider NTU Library
collection DR-NTU
language English
description We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data processing, purely absorptive 3D spectra of chlorophyll a are obtained.
author2 School of Physical and Mathematical Sciences
author_facet School of Physical and Mathematical Sciences
Zhang, Zhengyang
Wells, Kym Lewis
Tan, Howe-Siang
format Article
author Zhang, Zhengyang
Wells, Kym Lewis
Tan, Howe-Siang
spellingShingle Zhang, Zhengyang
Wells, Kym Lewis
Tan, Howe-Siang
Purely absorptive fifth-order three-dimensional electronic spectroscopy
author_sort Zhang, Zhengyang
title Purely absorptive fifth-order three-dimensional electronic spectroscopy
title_short Purely absorptive fifth-order three-dimensional electronic spectroscopy
title_full Purely absorptive fifth-order three-dimensional electronic spectroscopy
title_fullStr Purely absorptive fifth-order three-dimensional electronic spectroscopy
title_full_unstemmed Purely absorptive fifth-order three-dimensional electronic spectroscopy
title_sort purely absorptive fifth-order three-dimensional electronic spectroscopy
publishDate 2013
url https://hdl.handle.net/10356/99325
http://hdl.handle.net/10220/10942
_version_ 1759858294219866112

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