Purely absorptive fifth-order three-dimensional electronic spectroscopy

• Main Authors: Zhang, Zhengyang, Wells, Kym Lewis, Tan, Howe-Siang
• Other Authors: School of Physical and Mathematical Sciences
• Format: Article
• Language: English
• Published: 2013
• Online Access: https://hdl.handle.net/10356/99325; http://hdl.handle.net/10220/10942
• Institution: Nanyang Technological University

We demonstrate a method to measure a purely absorptive fifth-order three-dimensional (3D) electronic spectrum based on a pulse-shaper assisted pump-probe beam geometry setup. The 3D spectra are measured as a function of two independently controlled population times. With phase-cycling and data proce...